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Zhang, X, Hecobian, A, Zheng, M, Frank, NH, Weber, RJ (2010). "Biomass burning impact on PM2.5 over the southeastern US during 2007: integrating chemically speciated FRM filter measurements, MODIS fire counts and PMF analysis". ATMOSPHERIC CHEMISTRY AND PHYSICS, 10(14), 6839-6853.

Abstract
Archived Federal Reference Method (FRM) Teflon filters used by state regulatory agencies for measuring PM2.5 mass were acquired from 15 sites throughout the southeastern US and analyzed for water-soluble organic carbon (WSOC), water-soluble ions and carbohydrates to investigate biomass burning contributions to fine aerosol mass. Based on over 900 filters that spanned all of 2007, levoglucosan and K+ were studied in conjunction with MODIS Aqua fire count data to compare their performances as biomass burning tracers. Levoglucosan concentrations exhibited a distinct seasonal variation with large enhancement in winter and spring and a minimum in summer, and were well correlated with fire counts, except in winter when residential wood burning contributions were significant. In contrast, K+ concentrations had no apparent seasonal trend and poor correlation with fire counts. Levoglucosan and K+ only correlated well in winter (r(2) = 0.59) when biomass burning emissions were highest, whereas in other seasons they were not correlated due to the presence of other K+ sources. Levoglucosan also exhibited larger spatial variability than K+. Both species were higher in urban than rural sites (mean 44% higher for levoglucosan and 86% for K+). Positive Matrix Factorization (PMF) was applied to analyze PM2.5 sources and four factors were resolved: biomass burning, refractory material, secondary light absorbing WSOC and secondary sulfate/WSOC. The biomass burning source contributed 13% to PM2.5 mass annually, 27% in winter, and less than 2% in summer, consistent with other souce apportionment studies based on levoglucosan, but lower in summer compared to studies based on K+.

DOI:
10.5194/acp-10-6839-2010

ISSN:
1680-7316

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