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Panicker, AS, Pandithurai, G, Safai, PD, Kewat, S (2008). Observations of enhanced aerosol longwave radiative forcing over an urban environment. GEOPHYSICAL RESEARCH LETTERS, 35(4), L04817.

Abstract
Collocated measurements of sun/ sky radiance, aerosol chemical composition and radiative fluxes have been utilized to estimate longwave aerosol radiative forcing over Pune, an Indian urban site during dry winter [Dec2004 to Feb2005] by two methods. Hybrid method which uses observed downwelling and modeled upwelling longwave fluxes for different aerosol loadings yielded a surface forcing of 9.4 Wm(-2). Model approach includes utilization of skyradiometer derived spectral aerosol optical properties in the visible and near infra-red wavelengths, modeled aerosol properties in 1.2-40 mu m using observed soot and chemical composition data, MODIS water vapor and TOMS column ozone in a radiative transfer model. Estimates from model method showed longwave enhancement of 6.5 and 8.2Wm(-2) at the surface with tropical model atmosphere and temporally varying profiles of temperature and humidity, respectively. Study reveals that about 25% of the aerosol shortwave cooling is being compensated by increase in longwave radiation due to aerosol absorption.

DOI:
10.1029/2007GL032879

ISSN:
0094-8276

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