Publications

Kommula, SM; Buchholz, A; Gramlich, Y; Mielonen, T; Hao, L; Pullinen, I; Vettikkat, L; Ylisirni?, A; Joutsensaari, J; Schobesberger, S; Tiitta, P; Leskinen, A; Rees, DH; Haslett, SL; Siegel, K; Lunder, C; Zieger, P; Krejci, R; Romakkaniemi, S; Mohr, C; Virtanen, A (2024). Effect of Long-Range Transported Fire Aerosols on Cloud Condensation Nuclei Concentrations and Cloud Properties at High Latitudes. GEOPHYSICAL RESEARCH LETTERS, 51(6), e2023GL107134.

Abstract
Active vegetation fires in south-eastern (SE) Europe resulted in a notable increase in the number concentration of aerosols and cloud condensation nuclei (CCN) particles at two high latitude locations-the SMEAR IV station in Kuopio, Finland, and the Zeppelin Observatory in Svalbard, high Arctic. During the fire episode aerosol hygroscopicity kappa slightly increased at SMEAR IV and at the Zeppelin Observatory kappa decreased. Despite increased kappa in high CCN conditions at SMEAR IV, the aerosol activation diameter increased due to the decreased supersaturation with an increase in aerosol loading. In addition, at SMEAR IV during the fire episode, in situ measured cloud droplet number concentration (CDNC) increased by a factor of similar to 7 as compared to non-fire periods which was in good agreement with the satellite observations (MODIS, Terra). Results from this study show the importance of SE European fires for cloud properties and radiative forcing in high latitudes. Wildfires are large sources of aerosol particles and affect human health and climate. Aerosols from fires are transported long distances in the atmosphere and affect the aerosol and cloud properties at places far from the actual sources. In this study, we measured the long-range transported (LRT) fire air masses from south-eastern (SE) Europe at a northern European and a high Arctic site. LRT fire emissions from SE Europe increase the aerosol number and mass loading in Finland and even in the high Arctic. Results show that the effect of fire emissions on aerosol hygroscopicity depends on the properties of both the LRT fires and the background aerosols at a given location. The cloud properties analysis in eastern Finland shows that despite high hygroscopicity and increased CCN activity, the aerosol activation diameter for clouds increased during the fire episode. This is due to the depletion of available water vapor in clouds due to the increased aerosol loading. Satellite observations show an increase in cloud droplet number concentration during the fire episode confirming the effect of LRT fires on cloud properties in eastern Finland. This study can improve the understanding of the effect of LRT fires on aerosol and cloud properties at remote locations. Vegetation fires from southern Europe enhance aerosol and cloud condensation nuclei concentrations in northern Europe and the high Arctic A contrary trend in aerosol hygroscopicity is observed at these two locations during a strong fire episode as compared to non-fire periods Cloud droplet number concentrations in liquid clouds show strong response to fire aerosol both in in situ and satellite observations

DOI:
10.1029/2023GL107134

ISSN:
1944-8007